Simultaneous measurements of solid–liquid interfaces and bulk liquids using soft X-ray absorption spectroscopy

The Institute for Molecular Science, National Institutes of Natural Sciences
The Graduate University for Advanced Studies, SOKENDAI
High Energy Accelerator Research Organization, KEK

We have developed a method for making simultaneous soft X-ray absorption spectroscopy (XAS) measurements of solid-liquid interfaces and bulk liquids. By controlling the thickness of the liquid layer, we obtained the O K-edge XAS spectrum of bulk H2O from a liquid H2O layer on a thin Au film using the transmission method, and we used the electron-yield method to obtain the XAS spectrum of the H2O/Au interface by measuring the drain currents from the Au surface following soft X-ray absorption. This method for obtaining simultaneous XAS measurements of solid-liquid interfaces and bulk liquids can be utilized to investigate the mechanisms of a variety of catalytic, electrochemical, and biological reactions involving solid-liquid interfaces.

The experiments in this study were performed under the approval of the Photon Factory Program Advisory Committee (Proposal No. 2025S2-003).

Please refer to the website of the Institute for Molecular Science, National Institutes of Natural Sciences for details.

Contact

High Energy Accelerator Research Organization (KEK)
e-mail: press@kek.jp